ASTM E910-07(2013)

5.1 The HAFM test method is one of several available passive neutron dosimetry techniques (see, for example, Methods E854 and E1005). This test method can be used in combination with other dosimetry methods, or, if sufficient data are available from different HAFM sensor materials, as an alternative dosimetry test method. The HAFM method yields a direct measurement of total helium production in an irradiated sample. Absolute neutron fluence can then be inferred from this, assuming the appropriate spectrum integrated total helium production cross section. Alternatively, a calibration of the composite neutron detection efficiency for the HAFM method may be obtained by exposure in a benchmark neutron field where the fluence and spectrum averaged cross section are both known (see Matrix E706 IIE).

5.2 HAFMs have the advantage of producing an end product, helium, which is stable, making the HAFM method very attractive for both short-term and long-term fluence measurements without requiring time-dependent corrections for decay. HAFMs are therefore ideal passive, time-integrating fluence monitors. Additionally, the burnout of the daughter product, helium, is negligible.

5.3 The HAFM method is complementary to RM and solid state track recorder (SSTR) foils, and has been used as an integral part of the multiple foil method. The HAFM method follows essentially the same principle as the RM foil technique, which has been used successfully for accurate neutron dosimetry for the past 20 to 25 years. Various HAFM sensor materials exist which have significantly different neutron energy sensitivities from each other. HAFMs containing ¹⁰B and ⁶Li have been used routinely in LMFBR applications in conjunction with RM foils. The resulting data are entirely compatible with existing adjustment methods for radiometric foil neutron dosimetry (refer to Method E944).

5.4 An application for the HAFM method lies in the direct analysis of pressure vessel wall scrapings or Charpy block surveillance samples. Measurements of the helium production in these materials can provide in situ integral information on the neutron fluence spectrum. This application can provide dosimetry information at critical positions where conventional dosimeter placement is difficult if not impossible. Analyses must first be conducted to determine the boron, lithium, and other component concentrations, and their homogeneities, so that their possible contributions to the total helium production can be determined. Boron (and lithium) can be determined by converting a fraction of the boron to helium with a known thermal neutron exposure. Measurements of the helium in the material before and after the exposure will enable a determination of the boron content (7). Boron level down to less than 1 wt. ppm can be obtained in this manner.

5.5 By careful selection of the appropriate HAFM sensor material and its mass, helium concentrations ranging from ∼10⁻¹⁴ to 10⁻¹ atom fraction can be generated and measured. In terms of fluence, this represents a range of roughly 10¹² to 10²⁷ n/cm². Fluence (>1 MeV) values that may be encountered during routine surveillance testing are expected to range from ∼3 × 10¹⁴ to 2 × 10 ²⁰ n/cm², which is well within the range of the HAFM technique.

5.6 The analysis of HAFMs requires an absolute determination of the helium content. The analysis system specified in this test method incorporates a specialized mass spectrometer in conjunction with an accurately calibrated helium spiking system. Helium determination is by isotope dilution with subsequent isotope ratio measurement. The fact that the helium is stable makes the monitors permanent with the helium analysis able to be conducted at a later time, often without the inconvenience in handling caused by induced radioactivity. Such systems for analysis exist, and additional analysis facilities could be reproduced, should that be required. In this respect, therefore, the analytical requirements are similar to other ASTM test methods (compare with Test Method E244).